ARMA III definitely has more available for it in terms of special mods e.g. the canteen mod but also things like weapon sight swaying (something that annoys the hell out of me in most FPS games because it's usually vastly out of proportion to reality), weapon sight zoom (something else I find particularly annoying in FPS games is the crappy way that they implement using iron sights, the sights are typically too damned big for the sight picture and obscure the target, ARMA has usually been far better for this but the iron sights are often so small you can't see if you're actually on target!)
Plus they have all the other bits & pieces like firing from vehicles, towing vehicles and so on. That and the modding community is probably more active for ARMA III than it is for II, just look at the workshop on Steam, new mods are still being posted even as I type this!
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